The gamma-ray spectrum associated with the electron capture decay of 75Se has been studied with Ge(Li) spectrometers. Coincidence spectra were taken with a Ge(Li)Ge(Li) combination. The data do not support a recent report of several new gamma rays in the decay of 75Se. Gamma-gamma angular correlation experiments were performed with a NaI(Tl)Ge(Li) combination. The value obtained for δ(280 keV) is in excellent agreement with one recently reported value but in poor agreement with another. The ratio PK/Ptot for the electron capture branch to the 401 keV level of 75As has been determined, and the result agrees with previous experimental determinations. © 1969.