ENERGY-TRANSFER FROM AN EXCITED DYE MOLECULE TO THE SURFACE-PLASMONS OF AN ADJACENT METAL

被引:237
作者
WEBER, WH
EAGEN, CF
机构
[1] Physics Department, Research Staff, Ford Motor Company, Dearborn, MI
关键词
D O I
10.1364/OL.4.000236
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The probability for direct energy transfer from a dye molecule to the surface plasmons (SP) on a nearby metal is calculated using the classical Sommerfeld model. For 600-nm emission from a dipole-oriented ⊥ to an Ag surface, the peak SP coupling probability is 93% at a distance of 120 nm from the metal. The coupling is demonstrated in experiments with an Ag film between a rhodamine-methanol solution and a high-index prism. The SP-coupled radiation produces an intense cone of radiation in the prism, each frequency component of which satisfies the SP dispersion relation. © 1979, Optical Society of America.
引用
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页码:236 / 238
页数:3
相关论文
共 14 条
  • [1] Weber W.H., Eagen C.F., Bull. Am. Phys. Soc, 441, (1979)
  • [2] Sommerfeld A., Partial Differential Equations in Physics, (1949)
  • [3] Gerbshtein Y.M., merkulov I.A., Mirlin D.N., JETP Lett, 22, (1974)
  • [4] Benner R.E., Dornhaus R., pan C.A., Chang R.K., Bull. Am. Phys. Soc, 24, (1979)
  • [5] Otto A., Z. Phys, 216, (1968)
  • [6] Raether H., Physics of Thin Films, 9, (1977)
  • [7] Chance R.R., Prock A., Silbey R., Advances in Chemical Physics, XXXVII, (1978)
  • [8] Morawitz H., Philpott M.R., Phys. Rev., B 10, (1974)
  • [9] Philpott M.R., J. Chem. Phys, 62, (1975)
  • [10] Agarwal G.S., Phys. Rev, A 12, (1975)