GAS HOLD-UP, LIQUID CIRCULATION AND GAS-LIQUID MASS-TRANSFER IN SLURRY BUBBLE-COLUMNS

被引:0
|
作者
GAVROY, D [1 ]
JOLYVUILLEMIN, C [1 ]
CORDIER, G [1 ]
DELMAS, H [1 ]
机构
[1] RHONE POULENC,CNRS,UMR 45,F-69153 DECINES CHARPIEU,FRANCE
关键词
BUBBLE COLUMN; HYDRODYNAMICS; GAS HOLD-UP; MASS TRANSFER; HYDROGENATION; CATALYST LOADING;
D O I
暂无
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Hydrodynamic experiments have been performed with a small transparent piece of equipment. with and without an internal draft tube, operated at atmospheric pressure and room temperature. The effects of many parameters have been analysed separately: the role of the draft tube with various liquid phases (water, water-ethanol mixture and the reaction solvent) at various catalyst loadings. The overall gas hold-up is slightly reduced in the gas-lift operation, when compared to the simple bubble column. When varying the gas flow rate, the characteristic maximum of gas hold-up is only observed without the draft tube and for the ethanol-water mixture and the reaction solvent. The volumetric mass transfer coefficient has been determined in a very similar stainless steel reactor under pressure by two independent ways: a physical determination measuring dissolved hydrogen concentration variation with time and a chemical determination using a complete continuous reactor model including accurate reaction kinetics.
引用
收藏
页码:637 / 642
页数:6
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