Effect of the Electron Decay of Metallic Fission Products on the Chemical and Phase Compositions of an Uranium-Plutonium Fuel Irradiated by Fast Neutrons

被引：4

作者：

Bondarenko, G. G. ^{[1
]}

Bulatov, G. S. ^{[2
]}

Gedgovd, K. N. ^{[2
]}

Lyubimov, D. Yu. ^{[2
]}

Yakushkin, M. M. ^{[3
]}

机构：

[1] Res Inst Promising Mat & Technol, Moscow, Russia

[2] Russian Acad Sci, Inst Phys Chem & Electrochem, Moscow, Russia

[3] Tech Univ, Moscow Inst Elect & Math, Moscow, Russia

来源：

RUSSIAN METALLURGY | 2011年 / 11期

关键词：

D O I：

10.1134/S0036029511110036

中图分类号：

TF [冶金工业];

学科分类号：

0806 ;

摘要：

After fast-neutron irradiation, uranium-plutonium nitride U0.8Pu0.2N is shown to acquire a complex structure consisting of a solid solution that is based on the nitrides of uranium, plutonium, americium, neptunium, zirconium, yttrium, and lanthanides and contains condensed phases U2N3, CeRu2, BaTe, Ba3N2, CsI, Sr3N2, LaSe, metallic molybdenum, technetium, and U(Ru, Rh, Pd)(3) intermetallics. The contents and compositions of these phases are calculated at a temperature of 900 K and a burn-up fraction up to 14% (U + Pu). The change in the composition of the irradiated uranium-plutonium nitride is studied during the electron decay of metallic radionuclides. The kinetics of transformation of (URu3)-Ru-103, (CsI)-Cs-137, (Ba3N2)-Ba-140, and (PuN)-Pu-241 is calculated.

引用

页码：1074 / 1078

页数：5

共 18 条

[1]

[Anonymous], 2003, 020216463 RUSS FDN B

[2]

Bondarenko G. G., 2009, RUSSIAN METALLURGY M, P465

[3]

Bulatov G. S., 2009, MATERIALOVEDENIE, P2

[4]

GORBACHEV VM, 1976, INTERACTION RAD HEAV

[5]

Gurvich L. V., 1982, THERMODYNAMIC PROPER

[6]

Gusev N. G., 1988, RADIOACTIVE CHAINS H

[7]

Kiselev G V, 2001, ATOM TEKHN ZARUBEZH, P11

[8]

Kotelnikov R. B., 1978, HIGH TEMPERATURE NUC

[9] Prospects for the development of fast breeder reactors [J].

Mitenkov, FM .

ATOMIC ENERGY, 2002, 92 (06) :453-460

[10] Vaporization behavior of (Np,Pu)N [J].

Nakajima, K ;

Arai, Y ;

Suzuki, Y .

JOURNAL OF ALLOYS AND COMPOUNDS, 1998, 271 :666-669

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