CW ALL-OPTICAL TRIPLE RESONANCE SPECTROSCOPY

被引:55
作者
LYYRA, AM
WANG, H
WHANG, TJ
STWALLEY, WC
LI, L
机构
[1] CHINESE ACAD SCI,DALIAN INST CHEM PHYS,DALIAN,PEOPLES R CHINA
[2] UNIV IOWA HOSP & CLIN,DEPT PHYS & ASTRON,IOWA CITY,IA 52242
[3] UNIV IOWA HOSP & CLIN,DEPT CHEM,IOWA CITY,IA 52242
关键词
D O I
10.1103/PhysRevLett.66.2724
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
This paper reports for the first time continuous-wave, high-resolution, all-optical triple resonance spectroscopy. Using this technique, one can overcome the spin forbidden nature of a singlet-triplet transition and consequently unperturbed triplet rovibronic levels can be reached from a singlet ground state. This technique also facilitates state-selective population transfer to highly excited vibrational levels, both in the ground state and in excited states.
引用
收藏
页码:2724 / 2727
页数:4
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